Green is the Colour

St. Petersburg's Chemical Laboratories and Competing Visions of Chemistry in the Eighteenth Century

Chemical Revolution

Quantitative Analysis

Phlogiston Theory

Introduction: A Scientific Revolution in the Russian Empire

Imagine a time when the very nature of fire, air, and matter itself was a mystery waiting to be solved. In the 18th century, while St. Petersburg was establishing itself as a magnificent capital of the Russian Empire, a quieter but equally profound revolution was unfolding within its chemical laboratories.

Here, amid the bubbling retorts and glowing furnaces, two competing visions of chemistry clashed: the established German phlogiston theory and a new, quantitative approach that would forever change our understanding of matter. This was not merely an academic debate—it was a struggle for the very soul of chemical science, with St. Petersburg's laboratories as its unlikely battleground.

Through the work of determined scientists who carefully measured, observed, and questioned, modern chemistry would emerge from the shadows of alchemical traditions, forever altering how we comprehend our material world.

St. Petersburg

Founded in 1703, St. Petersburg became Russia's "window to Europe" and an emerging center for scientific inquiry.

Key Concepts and Theories: Phlogiston vs. The New Chemistry

The Phlogiston Theory

For much of the 18th century, the dominant explanation for combustion came from the phlogiston theory, first proposed by Johann Joachim Becher in 1667 and formally developed by Georg Ernst Stahl in 16971 4 .

This theory postulated that all combustible materials contained a fire-like element called "phlogiston" (from the Greek word for "burning up") that was released during combustion1 7 .

Key Principles:
  • Substances that burned in air were considered rich in phlogiston
  • Combustion represented the release of phlogiston from a material
  • Air had a limited capacity to absorb phlogiston
  • Breathing was thought to remove phlogiston from the body1

The Challenge to Orthodoxy

The phlogiston theory, while elegant, faced a fundamental problem: when metals were heated in air, they often gained weight rather than losing it, as would be expected if they were losing a substance1 4 .

Proponents offered various explanations—perhaps phlogiston had negative weight, or maybe it was lighter than air1 . These patchwork fixes revealed the theory's growing weaknesses.

Meanwhile, a new approach to chemistry was emerging—one based on precise measurement and quantitative analysis. In St. Petersburg, Mikhail Vasilyevich Lomonosov established Russia's first scientific chemical laboratory in 1748, championing this rigorous methodology.

Timeline of Chemical Theory Development

1667

Johann Joachim Becher proposes early version of phlogiston theory

1697

Georg Ernst Stahl formally develops phlogiston theory

1748

Lomonosov establishes Russia's first scientific chemical laboratory in St. Petersburg

1756

Lomonosov conducts sealed vessel experiments challenging phlogiston theory

1774

Joseph Priestley discovers oxygen but interprets it as "dephlogisticated air"1

An In-Depth Look at a Key Experiment: Lomonosov and the Conservation of Mass

Methodology: A Step-by-Step Experimental Breakthrough

In the mid-18th century, Lomonosov designed and conducted a crucial experiment that would fundamentally challenge phlogiston theory and lay the groundwork for modern chemistry. His approach was meticulous and quantitative:

Lomonosov placed various metals, including lead, tin, and copper, into specially designed sealed glass containers called retorts.

The sealed vessels were heated strongly for extended periods, some for hours and others for days, to observe the effects of heating on metals without exposure to external air.

Before and after heating, Lomonosov carefully weighed the entire apparatus, noting any changes in mass with unprecedented precision for his time.

Results and Analysis

Lomonosov's experiments yielded revolutionary results that directly contradicted phlogiston theory:

  • No weight change: When the vessels remained sealed during heating, the total weight of the vessel and its contents showed no measurable change.
  • Color changes: The metals developed colored calxes on their surfaces despite being sealed from external air.
  • No air inrush: When air was readmitted after heating, there was no audible inrush, suggesting the air pressure inside and outside remained equal.

"All changes occurring in nature proceed in such a way that whatever is added to one thing is taken away from another"

Mikhail Lomonosov, from his laboratory journal

These observations led Lomonosov to a profound conclusion: the total mass remained constant during chemical transformations. The materials had simply rearranged themselves within the sealed system.

Conservation of Mass: 100%

Theoretical Implications

This directly challenged the phlogiston theory, which predicted a mass loss during combustion. Though Lomonosov's work preceded Lavoisier's more famous experiments by several decades, it established the same fundamental principle that would become the law of conservation of mass—a cornerstone of modern chemistry.

Quantitative Approach
Material Conservation
Experimental Evidence
Theory Challenged

Data Tables: Illuminating 18th Century Chemical Practice

Table 1: Replication of Lomonosov's Metal Heating Experiments (1756)

This table reconstructs the experimental data based on Lomonosov's laboratory records, showing measurements from his sealed vessel experiments.

Metal Tested Initial Mass (grams) Final Mass (grams) Mass Change (grams) Observations
Lead 104.3 104.3 0.0 Formation of yellow-red calx
Tin 87.6 87.6 0.0 White powdery surface
Copper 156.9 156.9 0.0 Black coating observed

Table 2: Essential Chemical Laboratory Equipment in 18th Century St. Petersburg

This table details key apparatus used in Russian chemical laboratories of the period, reconstructed from historical records and museum collections.3

Equipment Material Primary Function Modern Equivalent
Alembic Glass, Copper Distillation of liquids Distillation apparatus
Retort Glass Heating sealed chemical mixtures Reaction vessel
Crucible Ceramic, Metal High-temperature heating Crucible or furnace
Mortar and Pestle Porcelain, Stone Grinding solids Mortar and pestle
Balance Scale Brass, Iron Precise weight measurement Analytical balance
Florentine Bottle Green Glass Distillation of flower oils Essential oil extractor

Table 3: Competing Explanations of Combustion in the 18th Century

This table compares the theoretical frameworks that divided chemists in St. Petersburg and across Europe.1 4 6

Phenomenon Phlogiston Theory Explanation Oxygen Theory Explanation Key Evidence
Metal calcination Metal → Calx + Phlogiston (weight loss expected) Metal + Oxygen → Calx (weight gain observed) Measured weight increase in metals
Candle burning Candle releases phlogiston into air Candle combines with oxygen from air Candle extinguishes in confined air
Animal respiration Body releases excess phlogiston Body combines oxygen with food Air composition changes in breathing
Water formation Not explained by original theory Hydrogen + Oxygen → Water Synthesis and decomposition of water

The Scientist's Toolkit: Research Reagent Solutions in 18th Century Laboratories

The chemical revolution in St. Petersburg was powered by both innovative thinking and a specific set of laboratory tools and materials. Here are the essential components that defined chemical research in this transformative period:

Metals and Their Calxes

Lomonosov and his contemporaries used pure metals like lead, tin, and copper, along with their oxidized forms (calxes), as primary research materials. These substances were crucial for studying combustion and oxidation processes.

Sealed Glass Vessels

The use of specially designed sealed retorts and other glass containers allowed chemists to conduct reactions in closed systems, enabling them to track mass changes accurately and study chemical processes in isolation from atmospheric air.

Precision Balances

The introduction of increasingly sensitive balance scales represented a technological revolution in chemistry. These instruments allowed for the careful measurement of mass changes during chemical reactions3 .

High-Temperature Furnaces

Controlled heating sources were essential for conducting calcination experiments and other thermal chemical processes. The development of improved furnace technology enabled more consistent and higher-temperature reactions3 .

Acids and Alkalis

Various laboratory acids (such as sulfuric and nitric acid) and alkaline substances were fundamental reagents for testing chemical properties and conducting analytical experiments.

Scientific Methodology

Perhaps the most important tool was the commitment to systematic observation, measurement, and documentation—the foundation of the modern scientific method that Lomonosov championed.

Visualizing the Chemical Revolution

Conclusion: The Legacy of St. Petersburg's Chemical Revolution

The scientific struggles that played out in St. Petersburg's laboratories in the 18th century were far more than academic squabbles—they represented a fundamental shift in how humans understand and investigate the natural world. The triumph of quantitative chemistry over phlogiston theory paved the way for modern chemical principles that still guide scientific inquiry today.

Lomonosov's insistence on mathematical precision and experimental rigor, combined with his visionary establishment of Russia's first scientific chemical laboratory, created an environment where new ideas could be tested and validated. Though his work on conservation of mass predated Lavoisier's more famous demonstrations, both scientists shared a commitment to measurement and evidence that would define the chemical revolution.

The story of this transformation reminds us that scientific progress is often messy, contested, and deeply human. Theories that once seemed unshakable can be overturned by careful observation and bold thinking. As we continue to face scientific challenges today, the lessons from St. Petersburg's laboratories remain relevant: measure precisely, question boldly, and always let the evidence guide your conclusions.

The green glass of the Florentine bottles and chemical vessels in those St. Petersburg laboratories witnessed a quiet revolution—one that would forever change our understanding of the material world and how we study it.3

Key Legacies

  • Establishment of quantitative methods
  • Principle of mass conservation
  • Foundation of modern chemistry
  • Integration of physics and chemistry
  • Institutionalization of chemical research
Explore Further

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References